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Selective Catalytic Hydrocarbons Oxidation: New Perspectives
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Editors: Ludmila I. Matienko, Larisa A. Mosolova and Gennady E. Zaikov (Emanuel Inst. of Biochemical Physic, Russian Academy of Sciences, Moscow, Russia)
Book Description:
The different methods for enhancing the catalytic activity of transition metal complexes in hydrocarbon (particularly, alkylarene) oxidations with dioxygen are briefly discussed. The role played by H-bonds in mechanisms of homogeneous catalysis is also analyzed. Furthermore, the authors propose a strategy of controlling the catalytic activity of Fe(II,III)(acac)n•L2 complexes (L2 = R4NBr or 18C6) by adding H2O to small concentrations. In addition, the activity of Ni, Fe, and Co catalysts in microsteps of chain initiation (O2 activation), and propagation (Cat + RO2•→) in the radical chain process of ethylbenzene oxidation is assessed by original method offered by authors. New concepts of mechanism of chain process of hydrocarbon oxidations with dioxygen, catalyzed with transition metal complexes, participation of catalysts in microsteps of complicated hydrocarbon oxidation, activity M-O2 (M = Co, Ni, Fe) complexes in different oxidation reactions are briefly stated, and the self-assembled (self-organized) systems mediated by transition metals are briefly considered in connection with increasing research interest in chemical transformations with use of these systems.

Table of Contents:
Preface pp. i-vii

Chapter I. Introduction, pp. 1-4

Chapter II. Homogeneous catalytic oxidations of alkylarens with molecular oxygen, pp. 5-6

Chapter III. The application of the different methods for increase in activity and selectivity of homogeneous catalysts in the oxidation processes, pp. 7-47

Chapter IV. The role of the Hydrogen–Bonding interactions in mechanisms of homogeneous catalysis, pp. 49-63

Chapter V. The mechanism of hydrocarbon liquid phase oxidation with dioxygen, catalyzed by complexes of transition metals, pp. 65-86

Chapter VI. Assessing active forms of iron and nickel catalysts in micro stages of radical-chain ethylbenzene oxidation, in the chain initiation (O2 activation), and propagation (Cat + RO2•→), pp. 87-108

Chapter VII. Catalytic oxidation of toluene and cumene in hydroperoxides in the presence of system {Ni(L1)2 + L2}, pp. 109-121

Chapter VIII. Self-Assembly and Self-Organized structures, mediated by transition metals, pp. 123-133

Chapter IX. Conclusion, pp. 135-149

Index pp. 151-158

   Binding: Hardcover
   Pub. Date: 2010
   Pages: 165, 6 x 9
   ISBN: 978-1-60876-385-6
   Status: AV
  
Status Code Description
AN Announcing
FM Formatting
PP Page Proofs
FP Final Production
EP Editorial Production
PR At Prepress
AP At Press
AV Available
  
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Selective Catalytic Hydrocarbons Oxidation: New Perspectives